 | Sean Connery | .... | Dr. Paul Bradley |
| Natalie Wood | .... | Tatiana Nikolaevna Donskaya |
| Karl Malden | .... | Harry Sherwood, NASA |
| Brian Keith | .... | Dr. Alexei Dubov |
| Martin Landau | .... | Major General Adlon |
| Trevor Howard | .... | Sir Michael Hughes |
| Richard Dysart | .... | Secretary of Defense |
| Henry Fonda | .... | The President |
| Joseph Campanella | .... | Lt. Gen. Easton |
| Bo Brundin | .... | Rolf Manheim |
| Katherine De Hetre | .... | Jan Watson |
| James G. Richardson | .... | Alan Marshall |
| Roger Robinson | .... | Bill Hunter |
| Michael Zaslow | .... | Sam Mason |
| John McKinney | .... | Peter Watson |
| John Findlater | .... | Astronaut Tom Easton |
| Paul Tulley | .... | Astronaut Bill Frager |
| Allen Williams | .... | Astronaut Michael McKendrick |
| Bibi Besch | .... | Helen Bradley |
| Gregory Gay | .... | Russian Premier |
| Clyde Kusatsu | .... | Yamashiro |
| Burke Byrnes | .... | Coast Guard Officer |
| Joe Medalis | .... | Bartender |
| Charles Bartlett | .... | Guard |
| Raymond O'Keefe | .... | Guard |
| Henry Olek | .... | Army Captain |
| Peter Bourne | .... | UN President |
| Stanley Mann | .... | Canadian U.N. Representative |
| Ronald Neame | .... | British U.N. Representative |
| Philip Sterling | .... | Russian U.N. Representative |
| Arthur Adams | .... | Ghana U.N. Representative |
| Fred Carney | .... | United States U.N. Representative |
| Sybil Danning | .... | Swiss Girl Skier |
| Meschino Paterlini | .... | Swiss Boy Skier |
| Jon Yune | .... | Siberian Man |
| Eileen Saki | .... | Siberian Woman |
| Chris Baur | .... | Communications Center Technician |
| Paul Camen | .... | Communications Center Technician |
| Dorothy Catching | .... | Communications Center Technician |
| Bill Couch | .... | Communications Center Technician |
| William Darr | .... | Communications Center Technician |
| Joan Foley | .... | Communications Center Technician |
| Paul L. Ehrmann | .... | Communications Center Technician |
| Johnny Moio | .... | Communications Center Technician |
| Read Morgan | .... | Communications Center Technician |
| Conrad Palmisano | .... | Communications Center Technician |
| Tony Rocco | .... | Communications Center Technician |
| Jesse Wayne | .... | Communications Center Technician |
| Carole Hemingway | .... | Gladys, Sherwood's Secretary |
| Clete Roberts | .... | Network Newscaster |
| Stu Nahan | .... | Football Announcer |
| Osman Ragheb | .... | Osman Ragheb |
| Yang Yu | .... | Chinese Fisherman |
| Yau Tsui Ling | .... | Chinese Fisherman's Wife |
| Rick Slaven | .... | Canteen Worker |
| James Bacon | .... | News Reporter |
| Yani Begakis | .... | News Reporter |
| Selma Archerd | .... | Woman in Subway |
| Domingo Ambriz | .... | Boy with Radio |
| Peter Donat | .... | Opening Sequence Narrator (Stimme) |
| Simon Cadell | .... | BBC News Reporter (uncredited) |
| George Golden | .... | U.N. meeting attendee (uncredited) |
| Wei Tu Lin | .... | Escaping tenant (uncredited) |
| Tony Regan | .... | U.N. meeting attendee (uncredited) |
| John Spencer | .... | Control center worker (uncredited) |
| Arthur Tovey | .... | U.N. meeting attendee (uncredited) |
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